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Core Capabilities & Methodology

Materials Discovery, Synthesis & Characterisation

Pioneering scalable chemical synthesis, defect engineering, and operando synchrotron diagnostics to discover next-generation semiconductor materials for clean energy systems.

The Research Trinity

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High-Throughput Synthesis

Precision solution-based synthesis of halide perovskites, 2D MXenes, and nanostructured metal oxides in inert glovebox lines.

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Defect & Interface Engineering

Chemical passivation and composition tuning to eliminate trap states, improve carrier transport, and enhance long-term stability.

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Operando & Synchrotron Diagnostics

Advanced structural and optical characterisation tracking film crystallisation and degradation dynamics in real time.

Featured Research Thrusts 

Halide Perovskites and
Lead-Free Semiconductors

Author et al., Perovskite Paper 1 (Year)

Journal Name [ DOI Link - ]

Author et al., Perovskite Paper 2 (Year)
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Author et al., Perovskite Paper 3 (Year)

Author et al., Perovskite Paper 4 (Year)

Halide Perovskites & Emerging Lead-Free Semiconductors

Research Scope: We investigate lead-halide perovskites, low-dimensional perovskites, and lead-free alternatives (such as bismuth/copper-based quaternary halides) for optoelectronic and energy applications.

Focus & Applications: Addressing operational stability, moisture tolerance, defect passivation, and environmental toxicity—paving the way for sustainable deployment in indoor photovoltaics, consumer electronics, and wireless IoT networks.

Nanostructured Oxides, 2D Materials & Molecular Complexes

Research Scope: Beyond traditional semiconductors, we synthesise and tune nanostructured metal oxides, 2D layered double hydroxides (LDHs), and molecular complexes (e.g., cobalt phthalocyanines).

Focus & Applications: By controlling local coordination, stoichiometry, and heterojunction interfaces, we engineer these materials for high-performance electrocatalytic water splitting, green hydrogen generation, and CO₂ reduction.

Nanostructured
Oxides and 2D Materials

Author et al., Electrocatalysis Paper 1 (Year)
Journal Name [ DOI Link - ]

Author et al., Electrocatalysis Paper 2 (Year)
Journal Name [ DOI Link - ]

Author et al., Electrocatalysis Paper 3 (Year)

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Author et al., Synchrotron Paper 1 (Year)
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Author et al., Synchrotron Paper 2 (Year)
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Author et al., Synchrotron Paper 3 (Year)

Author et al., Synchrotron Paper 4 (Year)

Advanced Synchrotron & Spectroscopic Diagnostics

Research Scope: To unearth structure-property-function relationships, we leverage cutting-edge characterisation methods, including synchrotron-based techniques at the Diamond Light Source.

Key Techniques: Using methods such as Grazing-Incidence Wide-Angle X-ray Scattering (GIWAXS) and Hard X-ray Photoelectron Spectroscopy (HAXPES), we probe film morphology, buried interfaces, crystallographic orientation, and electronic surface states at atomic precision.

Fundamental Photophysics, Photodoping & Photon Recycling

Research Scope: We explore light-matter interactions and carrier transport dynamics across advanced semiconductor thin films.

Focus & Applications: Our studies focus on passivating monovalent cation/halide additives (e.g., K⁺, Rb⁺), understanding photodoping mechanisms, controlling local charge-carrier accumulation, and harnessing photon recycling to maximise photoluminescence quantum efficiency and photovoltaic power conversion.

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Author et al., Photophysics Paper 1 (Year)
Journal Name [ DOI Link - ]

 Author et al., Photophysics Paper 2 (Year)
Journal Name [ DOI Link - ]

Author et al., Photophysics Paper 3 (Year)

Featured Research Thrusts 

Nitrogen Glovebox Lines

Solar Simulators (Class AAA)

In-situ PL Mapping

Spin-Coaters & Blade Coaters

Atomic Layer Deposition

Electrocatalytic Cells

Collaborate on Materials Discovery

Interested in partnering on advanced characterisation, testing materials, or pursuing doctoral/postdoctoral research at UCL?

Related Publications

01
Photodoping through local charge carrier accumulation in alloyed hybrid perovskites for highly efficient luminescence

S. Feldmann, M. Abdi-Jalebi, et al., R. H. Friend, F. Deschler. Nature Photonics, 14, 123–128 (2020).

02
Lanthanide-doped inorganic nanoparticles turn molecular triplet excitons bright

S. Han, M. Abdi-Jalebi, et al., A. Rao. Nature, 587, 594–599 (2020).

03
Photon recycling in lead iodide perovskite solar cells

L. M. Pazos-Outón, M. Abdi-Jalebi, et al., R. H. Friend, F. Deschler. Science, 351, 1430–1433 (2016).

04
Potassium- and Rubidium-Passivated Alloyed Perovskite Films: Optoelectronic Properties and Moisture Stability

M. Abdi-Jalebi, et al., R. H. Friend, S. D. Stranks. ACS Energy Letters, 3, 2671–2678 (2018)

05
Highly Absorbing Lead-Free Semiconductor Cu₂AgBiI₆ for Photovoltaic Applications from the Quaternary CuI–AgI–BiI₃ Phase Space

H. C. Sansom, M. Abdi-Jalebi, et al., L. M. Herz, H. J. Snaith, M. J. Rosseinsky. Journal of the American Chemical Society, 143 (10), 3983–3992 (2021)

06
Growth Engineering of CH₃NH₃PbI₃ Structures for High-Efficiency Solar Cells

M. I. Dar, M. Abdi-Jalebi, N. Arora, M. Grätzel, M. K. Nazeeruddin. Advanced Energy Materials, 6, 1501358 (2016).

07
Impact of Monovalent Cation Halide Additives on the Structural and Optoelectronic Properties of CH₃NH₃PbI₃ Perovskite

M. Abdi-Jalebi, et al., M. Grätzel, R. H. Friend. Advanced Energy Materials, 6, 1502472 (2016)

08
Recent progress in morphology optimization in perovskite solar cell

N. K. Tailor, M. Abdi-Jalebi, et al., S. Satapathi. Journal of Materials Chemistry A, 8, 21356–21386 (2020).

Key Research Directions

One of our primary research focuses is halide perovskites, a highly promising class of materials for next-generation high-performance optoelectronic devices, including solar cells and light-emitting diodes (LEDs). These materials challenge conventional understanding by exhibiting exceptional optoelectronic properties—such as strong light absorption and long charge-carrier diffusion lengths—despite having moderate defect densities. As a result, perovskite solar cells have achieved power conversion efficiencies (PCEs) exceeding 25%. While remarkable progress has been made over the past decade, the widespread adoption of perovskite-based energy technologies requires major advances in material stability, long-term operational lifetime, and environmental sustainability. Developing non-toxic alternatives is also essential for enabling applications in wireless sensor networks, consumer electronics, and Internet of Things (IoT) devices. Our research explores scalable synthesis methods for a wide range of halide perovskites and other advanced semiconductors. We investigate their structural and optoelectronic properties, including thin-film morphology, compositional engineering, charge-carrier dynamics, and photon recycling. In addition, we utilize advanced synchrotron characterization techniques at the Diamond Light Source, including Grazing-Incidence Wide-Angle X-ray Scattering (GIWAXS) and Hard X-ray Photoelectron Spectroscopy (HAXPES), to gain deeper insights into semiconductor materials and device performance.

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Representative Publications

[1] M Ibrahim Dar, Mojtaba Abdi‐Jalebi, Neha Arora, Michael Grätzel, Mohammad Khaja Nazeeruddin; “Growth Engineering of CH3NH3PbI3 Structures for High‐Efficiency Solar Cells” Adv. Energy Mater.  6, 1501358 (2016).

[2] Mojtaba Abdi-Jalebi, et al., Michael Grätzel, Richard H. Friend; “Impact of Monovalent Cation Halide Additives on the Structural and Optoelectronic Properties of CH3NH3PbI3 Perovskite” Adv. Energy Mater., 6, 1502472 (2016).

[3] Sanyang Han, et al., Mojtaba Abdi-Jalebi, Akshay Rao, “Lanthanide-doped inorganic nanoparticles turn molecular triplet excitons bright”, Nature, 587, 594–599 (2020).

[4] Naveen Kumar Tailor, Mojtaba Abdi-Jalebi, et al., Soumitra Satapathi, “Recent progress in morphology optimization in perovskite solar cell”, J. Mater. Chem. A, 2020,8, 21356-21386.

[5] Mojtaba Abdi-Jalebi, et al., Richard H. Friend, Samuel D. Stranks, “Potassium- and Rubidium-Passivated Alloyed Perovskite Films: Optoelectronic Properties and Moisture Stability”, ACS Energy Lett., 3, pp 2671–2678 (2018).

[6] Harry C Sansom, et al., Mojtaba Abdi-Jalebi, Laura M Herz, Henry J Snaith, Matthew J Rosseinsky, “Highly Absorbing Lead-Free Semiconductor Cu2AgBiI6 for Photovoltaic Applications from the Quaternary CuI–AgI–BiI3 Phase Space”, J. Am. Chem. Soc., 143, 10, 3983–3992 (2021).

[7] Sascha Feldmann, Mojtaba Abdi-Jalebi, et al., Felix Deschler, “Photodoping through local charge carrier accumulation in alloyed hybrid perovskites for highly efficient luminescence”, Nature Photonics, 14, 123–128 (2020).

[8] Luis Pazos-Outón, Mojtaba Abdi-Jalebi, et al., Richard Friend, Felix Deschler, “Photon recycling in lead iodide perovskite solar cells” Science, 351, 1430-1433 (2016).

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